A Polar Corundum Oxide Displaying Weak Ferromagnetism at Room Temperature

نویسندگان

  • Man-Rong Li
  • Umut Adem
  • Sean R. C. McMitchell
  • Zhongling Xu
  • Chris I. Thomas
  • John E. Warren
  • Duong V. Giap
  • Hongjun Niu
  • Xinming Wan
  • Robert G. Palgrave
  • Florian Schiffmann
  • Furio Cora
  • Ben Slater
  • Tim L. Burnett
  • Markys G. Cain
  • Artem M. Abakumov
  • Gustaaf van Tendeloo
  • Michael F. Thomas
  • Matthew J. Rosseinsky
  • John B. Claridge
چکیده

Combining long-range magnetic order with polarity in the same structure is a prerequisite for the design of (magnetoelectric) multiferroic materials. There are now several demonstrated strategies to achieve this goal, but retaining magnetic order above room temperature remains a difficult target. Iron oxides in the +3 oxidation state have high magnetic ordering temperatures due to the size of the coupled moments. Here we prepare and characterize ScFeO(3) (SFO), which under pressure and in strain-stabilized thin films adopts a polar variant of the corundum structure, one of the archetypal binary oxide structures. Polar corundum ScFeO(3) has a weak ferromagnetic ground state below 356 K-this is in contrast to the purely antiferromagnetic ground state adopted by the well-studied ferroelectric BiFeO(3).

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عنوان ژورنال:

دوره 134  شماره 

صفحات  -

تاریخ انتشار 2012